Ex situ mineral carbonation for CO2 mitigation: Evaluation of mining waste resources, aqueous carbonation processability and life cycle assessment (Carmex project) - Archive ouverte HAL Accéder directement au contenu
Article Dans Une Revue Minerals Engineering Année : 2014

Ex situ mineral carbonation for CO2 mitigation: Evaluation of mining waste resources, aqueous carbonation processability and life cycle assessment (Carmex project)

(1) , (2) , (3) , (1) , (2) , (2) , (4) , (3) , (1) , (1) , (5) , (5)
1
2
3
4
5

Résumé

This article presents the main outputs from the multidisciplinary Carmex project (2009-2012), which was concerned with the possibility of applying ex situ mineral carbonation concepts to mafic/ultramafic mining wastes. Focus points of the project included (i) matching significant and accessible mining wastes to large CO2 emitters through a dedicated geographical information system (GIS), (ii) analysis of aqueous carbonation mechanisms of mining waste and process development and (iii) environmental assessment of ex situ mining waste carbonation through life cycle assessment (LCA) methodology. With a number of materials associated with the mining sector, the project took a close look at the aqueous carbonation mechanisms for these materials and obtained unexpected carbonation levels (up to 80%) by coupling mechanical exfoliation and reactive carbonation. Results from this work support the possibility of processing serpentine-rich peridotites without applying the classical first step of heat activation. Perspectives are also given for the carbonation of Ni-pyrometallurgical slag available closed to ultramafic mining residues. LCA of the mining waste carbonation system as a whole made it clear that the viability of this CO2 storage option lies with the carbonation process itself and optimisation of its operating conditions. By combining the body of knowledge acquired by this project, it is concluded that New Caledonia, with its insularity and local abundance of 'carbonable' rocks and industrial wastes coupled with significant greenhouse gas (GHG) emissions from world-class nickel pyro and hydrometallurgical industries stands out as a strong potential candidate for application of ex situ mineral carbonation.
Fichier principal
Vignette du fichier
20140512110136749.pdf (4.84 Mo) Télécharger le fichier
Origine : Fichiers produits par l'(les) auteur(s)

Dates et versions

hal-00987658 , version 1 (12-05-2014)

Identifiants

Citer

Françoise Bodénan, Florent Bourgeois, Charlotte Petiot, Thierry Augé, Benjamin Bonfils, et al.. Ex situ mineral carbonation for CO2 mitigation: Evaluation of mining waste resources, aqueous carbonation processability and life cycle assessment (Carmex project). Minerals Engineering, 2014, 59, pp.52-63. ⟨10.1016/j.mineng.2014.01.011⟩. ⟨hal-00987658⟩
708 Consultations
654 Téléchargements

Altmetric

Partager

Gmail Facebook Twitter LinkedIn More